Sorry to hear this... Oyster shell scale is the king pin of the scale world... That shell makes them almost immune to many pesticides. In this case, you are definitely doing it right by removing as many as you can see. Keep removing and then spray. You might have to do 2-3 spraying and removal sessions that are about 3 weeks apart each.
Here is something I posted in response to a juniper scale issue. I have never used this on pines. However, I would imagine it would not hurt the pine.
I have been dealing with scale on junipers for almost 10 years. I will offer this. The home made solution works very well. You will have to spray a couple of times probably every season, but it is worth it. Especially at the very end of winter.
These are the general ratios. You can use a little more oil and you can use as much as 2 tablespoons of soap for bad infestations.
1 tablespoon of vegetable oil
1 1/2 tablesspoons of dishwashing liquid. You can use palmolive or ivory. I have used both.
Mix this in a gallon of water. Then pour this solution in a spray bottle. Now add 1 capful (from the alcohol bottle) of alcohol. Shake well. Spay all surfaces, under and over branches, interiors, trunk etc..I usually leave it on for about 24 hours then shower the tree off very well. In a few weeks, I'll sometimes repeat it again. I would not spray in temps that are below freezing or above 90. However, you can offer some protection for the trees anyway. After spraying, I usually keep the tree out of direct sun for a few days and after the tree is thoroughly hosed off.
I also had success with Bonide all seasons horticultural oil years ago. However, I switched to this because it is not toxic at all. It can be sprayed inside, outside and no PPE in necessary.
Rob