a treatment will take weeks to correct an imbalance, Fe deficient trees will show speckling and chlorosis; these are not symptoms of your Fe treatment. Especially because you have not corrected the pH issue yet; The black dots are probably localized necrosis; areas of immediate cell death.
I would guess that the leaf curl is from nutrient burn. If you used a lot of Fe it will cause the absorption of more nutrients than are normally possible. Do the leafs feel brittle and thin, like burnt news-paper?
I would do the following:
remove from the pot and assess the roots; if you see white new growth you'll probably be ok to do the following - gently comb out the exterior roots of the root ball with your FINGERS. This means lightly unwind the new growth, saving and protecting all the little new root hairs. Do not try to break up the root ball, your aim is to loosen it as best you can without breaking or damaging the roots (this is nearly impossible to not cause some sort of damage) Then repot into a bigger container with free-draining soil. I'd recommend 80 % perlite 10% peat and 10% sand. Leave all the old soil on the root ball until next year.
If the roots are a black mushy mess; gently remove the dead mushy roots as best you can - they are not helping anything and may only cause further rot. then pot in larger container as described above.
I'd do this to promote new root growth into free draining substrate. this will allow you to water more frequently, as the tree comes back to health.
You need to lower your pH, 6.5 is good, do not go below 6.2 or other macro nutrient may become toxic in your soil. chelated Fe becomes toxic at pH 5.8 and below. fill up a trash can or buckey with water daily - fluoride and chloride will evaporate out of solution if you can let your water sit for 2-3 days before using it, adjust your pH before watering. Do not add nutrients into the water reservoir until your ready to feed your tree. Don't feed your tree until new healthy growth is visible. a solution of peroxide may help; use as directed (1 tbs 3% H2O2 per gallon) the oxidizing effect will kill rot causing fungus and provide oxygen to your starved root system. Again, this is if you find the roots in poor health; watering with H2O2 is a remedy for over watered plants; its a way to deliver oxygen to drowning roots.
aeration of the soil, gentile Fe application (I believe twice a year as directed is all you need, you already did one), free draining soil.